Migration of Per‐ and Polyfluoroalkyl Substances in Soil Under Rainfall Simulation.
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| Title: | Migration of Per‐ and Polyfluoroalkyl Substances in Soil Under Rainfall Simulation. |
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| Authors: | Liang, Minshu1 (AUTHOR) minshu.liang@adelaide.edu.au, Kabiri, Shervin1 (AUTHOR), McLaughlin, Michael J.1 (AUTHOR), Navarro, Divina2 (AUTHOR) |
| Source: | CLEAN: Soil, Air, Water. Apr2026, Vol. 54 Issue 4, p1-10. 10p. |
| Subject Terms: | *Runoff, *Leaching, *Soil moisture, *Soil pollution, Rainfall simulators, Evaporative power, Fluoroalkyl compounds |
| Abstract: | Understanding the migration of per‐ and polyfluoroalkyl substances (PFAS) in soil via groundwater and surface water is vital for managing PFAS. PFAS transport via surface runoff during rainfall is less known than leaching. This study investigated PFAS migration under simulated rainfall in soils with varying contamination levels, examining multiple pathways to assess the factors affecting PFAS migration. Rainfall simulations were conducted over 15 days with wetting and drying cycles. Results indicate that leaching is likely the dominant pathway for PFAS transport, accounting for the largest proportion (on average 72%) of PFAS mass in the released fractions. Runoff was also an important pathway for long‐chain PFAS, whereas short‐chain PFAS were not detected in runoff. Both PFAS concentration and the wetting‐drying cycles influenced PFAS distribution. Leaching was negligible when PFAS concentrations exceeded 30 mg/kg perfluorooctane sulfonic acid (PFOS), potentially due to reduction in soil hydraulic conductivity. PFAS concentrations in runoff increased following extended drying periods, suggesting accumulation of PFAS in the upper soil. This pattern of evapoconcentration, likely driven by capillary water movement and subsequent evaporation, is consistent with the resurgence of concentration in surface soils. Overall results highlight that surface runoff is an important pathway for PFAS transport, particularly for long chain PFAS. Wetting and drying cycles may promote accumulation in the upper soil layers, increasing the potential for mobilization via runoff. By considering both leaching and runoff, this study contributes to a better understanding of PFAS transport in soils and can help inform management strategies to reduce contaminant spread to surface waters. [ABSTRACT FROM AUTHOR] |
| Copyright of CLEAN: Soil, Air, Water is the property of Wiley-Blackwell and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.) | |
| Database: | GreenFILE |
| FullText | Text: Availability: 0 |
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| Header | DbId: 8gh DbLabel: GreenFILE An: 193163294 AccessLevel: 6 PubType: Academic Journal PubTypeId: academicJournal PreciseRelevancyScore: 0 |
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| Items | – Name: Title Label: Title Group: Ti Data: Migration of Per‐ and Polyfluoroalkyl Substances in Soil Under Rainfall Simulation. – Name: Author Label: Authors Group: Au Data: <searchLink fieldCode="AR" term="%22Liang%2C+Minshu%22">Liang, Minshu</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> minshu.liang@adelaide.edu.au</i><br /><searchLink fieldCode="AR" term="%22Kabiri%2C+Shervin%22">Kabiri, Shervin</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22McLaughlin%2C+Michael+J%2E%22">McLaughlin, Michael J.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Navarro%2C+Divina%22">Navarro, Divina</searchLink><relatesTo>2</relatesTo> (AUTHOR) – Name: TitleSource Label: Source Group: Src Data: <searchLink fieldCode="JN" term="%22CLEAN%3A+Soil%2C+Air%2C+Water%22">CLEAN: Soil, Air, Water</searchLink>. Apr2026, Vol. 54 Issue 4, p1-10. 10p. – Name: Subject Label: Subject Terms Group: Su Data: *<searchLink fieldCode="DE" term="%22Runoff%22">Runoff</searchLink><br />*<searchLink fieldCode="DE" term="%22Leaching%22">Leaching</searchLink><br />*<searchLink fieldCode="DE" term="%22Soil+moisture%22">Soil moisture</searchLink><br />*<searchLink fieldCode="DE" term="%22Soil+pollution%22">Soil pollution</searchLink><br /><searchLink fieldCode="DE" term="%22Rainfall+simulators%22">Rainfall simulators</searchLink><br /><searchLink fieldCode="DE" term="%22Evaporative+power%22">Evaporative power</searchLink><br /><searchLink fieldCode="DE" term="%22Fluoroalkyl+compounds%22">Fluoroalkyl compounds</searchLink> – Name: Abstract Label: Abstract Group: Ab Data: Understanding the migration of per‐ and polyfluoroalkyl substances (PFAS) in soil via groundwater and surface water is vital for managing PFAS. PFAS transport via surface runoff during rainfall is less known than leaching. This study investigated PFAS migration under simulated rainfall in soils with varying contamination levels, examining multiple pathways to assess the factors affecting PFAS migration. Rainfall simulations were conducted over 15 days with wetting and drying cycles. Results indicate that leaching is likely the dominant pathway for PFAS transport, accounting for the largest proportion (on average 72%) of PFAS mass in the released fractions. Runoff was also an important pathway for long‐chain PFAS, whereas short‐chain PFAS were not detected in runoff. Both PFAS concentration and the wetting‐drying cycles influenced PFAS distribution. Leaching was negligible when PFAS concentrations exceeded 30 mg/kg perfluorooctane sulfonic acid (PFOS), potentially due to reduction in soil hydraulic conductivity. PFAS concentrations in runoff increased following extended drying periods, suggesting accumulation of PFAS in the upper soil. This pattern of evapoconcentration, likely driven by capillary water movement and subsequent evaporation, is consistent with the resurgence of concentration in surface soils. Overall results highlight that surface runoff is an important pathway for PFAS transport, particularly for long chain PFAS. Wetting and drying cycles may promote accumulation in the upper soil layers, increasing the potential for mobilization via runoff. By considering both leaching and runoff, this study contributes to a better understanding of PFAS transport in soils and can help inform management strategies to reduce contaminant spread to surface waters. [ABSTRACT FROM AUTHOR] – Name: AbstractSuppliedCopyright Label: Group: Ab Data: <i>Copyright of CLEAN: Soil, Air, Water is the property of Wiley-Blackwell and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.) |
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| RecordInfo | BibRecord: BibEntity: Identifiers: – Type: doi Value: 10.1002/clen.70161 Languages: – Code: eng Text: English PhysicalDescription: Pagination: PageCount: 10 StartPage: 1 Subjects: – SubjectFull: Runoff Type: general – SubjectFull: Leaching Type: general – SubjectFull: Soil moisture Type: general – SubjectFull: Soil pollution Type: general – SubjectFull: Rainfall simulators Type: general – SubjectFull: Evaporative power Type: general – SubjectFull: Fluoroalkyl compounds Type: general Titles: – TitleFull: Migration of Per‐ and Polyfluoroalkyl Substances in Soil Under Rainfall Simulation. Type: main BibRelationships: HasContributorRelationships: – PersonEntity: Name: NameFull: Liang, Minshu – PersonEntity: Name: NameFull: Kabiri, Shervin – PersonEntity: Name: NameFull: McLaughlin, Michael J. – PersonEntity: Name: NameFull: Navarro, Divina IsPartOfRelationships: – BibEntity: Dates: – D: 01 M: 04 Text: Apr2026 Type: published Y: 2026 Identifiers: – Type: issn-print Value: 18630650 Numbering: – Type: volume Value: 54 – Type: issue Value: 4 Titles: – TitleFull: CLEAN: Soil, Air, Water Type: main |
| ResultId | 1 |