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Highly Efficient Binuclear Copper‐catalyzed Oxidation of N,N‐Dimethylanilines with O2.

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Title: Highly Efficient Binuclear Copper‐catalyzed Oxidation of N,N‐Dimethylanilines with O2.
Authors: Liu, Yuxia1 (AUTHOR) yuxialiu@nwu.edu.cn, Yan, Yonggang2 (AUTHOR), Xue, Dong2 (AUTHOR), Wang, Zhongfu1 (AUTHOR), Xiao, Jianliang2,3 (AUTHOR), Wang, Chao2 (AUTHOR) c.wang@snnu.edu.cn
Source: ChemCatChem. 4/20/2020, Vol. 12 Issue 8, p2221-2225. 5p.
Subjects: Oxidation, Homogeneous catalysis
Abstract: A binuclear copper‐salicylate complex, [Cu(Sal)2(NCMe)]2 (Sal=salicylate), was found to be an active catalyst for the oxidation of N,N‐dimethylanilines by O2, affording the corresponding N‐methyl‐N‐phenylformamides as major products. The reactions were carried out with a O2 balloon and the S/C (substrate/catalyst ratio) of the model reaction could be up to 1×105, providing a practical and highly efficient catalytic protocol for accessing N‐methyl‐N‐phenylformamides. [ABSTRACT FROM AUTHOR]
Copyright of ChemCatChem is the property of Wiley-Blackwell and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
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  Data: Highly Efficient Binuclear Copper‐catalyzed Oxidation of N,N‐Dimethylanilines with O<subscript>2</subscript>.
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  Data: <searchLink fieldCode="AR" term="%22Liu%2C+Yuxia%22">Liu, Yuxia</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> yuxialiu@nwu.edu.cn</i><br /><searchLink fieldCode="AR" term="%22Yan%2C+Yonggang%22">Yan, Yonggang</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Xue%2C+Dong%22">Xue, Dong</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Wang%2C+Zhongfu%22">Wang, Zhongfu</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Xiao%2C+Jianliang%22">Xiao, Jianliang</searchLink><relatesTo>2,3</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Wang%2C+Chao%22">Wang, Chao</searchLink><relatesTo>2</relatesTo> (AUTHOR)<i> c.wang@snnu.edu.cn</i>
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  Data: <searchLink fieldCode="JN" term="%22ChemCatChem%22">ChemCatChem</searchLink>. 4/20/2020, Vol. 12 Issue 8, p2221-2225. 5p.
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  Data: <searchLink fieldCode="DE" term="%22Oxidation%22">Oxidation</searchLink><br /><searchLink fieldCode="DE" term="%22Homogeneous+catalysis%22">Homogeneous catalysis</searchLink>
– Name: Abstract
  Label: Abstract
  Group: Ab
  Data: A binuclear copper‐salicylate complex, [Cu(Sal)2(NCMe)]2 (Sal=salicylate), was found to be an active catalyst for the oxidation of N,N‐dimethylanilines by O2, affording the corresponding N‐methyl‐N‐phenylformamides as major products. The reactions were carried out with a O2 balloon and the S/C (substrate/catalyst ratio) of the model reaction could be up to 1×105, providing a practical and highly efficient catalytic protocol for accessing N‐methyl‐N‐phenylformamides. [ABSTRACT FROM AUTHOR]
– Name: AbstractSuppliedCopyright
  Label:
  Group: Ab
  Data: <i>Copyright of ChemCatChem is the property of Wiley-Blackwell and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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        Value: 10.1002/cctc.201901962
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      – Code: eng
        Text: English
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      – SubjectFull: Homogeneous catalysis
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      – TitleFull: Highly Efficient Binuclear Copper‐catalyzed Oxidation of N,N‐Dimethylanilines with O2.
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            NameFull: Yan, Yonggang
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            – D: 20
              M: 04
              Text: 4/20/2020
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              Y: 2020
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