Spectroscopic study and lifetime measurement of the 6d7p3F2o state of radium.

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Title: Spectroscopic study and lifetime measurement of the 6d7p3F2o state of radium.
Authors: Booth, D.W.1 (AUTHOR) dbooth@anl.gov, Rabga, T.1,2 (AUTHOR), Ready, R.2 (AUTHOR), Bailey, K.G.1 (AUTHOR), Bishof, M.1 (AUTHOR), Dietrich, M.R.1 (AUTHOR), Greene, J.P.1 (AUTHOR), Mueller, P.1 (AUTHOR), O'Connor, T.P.1 (AUTHOR), Singh, J.T.2 (AUTHOR)
Source: Spectrochimica Acta Part B. Oct2020, Vol. 172, pN.PAG-N.PAG. 1p.
Subjects: Oscillator strengths, Spin-orbit interactions, Atomic beams, Radium, Branching ratios, Metastable states
Abstract: We report a method for the precision measurement of the oscillator strengths and the branching fractions of the decay channels of the 6 d 7 p 3 F 2 o state in 226Ra. This method exploits a set of metastable states present in Ra, allowing a measurement of the oscillator strengths that does not require knowledge of the number of atoms in the atomic beam. We measure the oscillator strengths and the branching fractions for decays from the 6 d 7 p 3 F 2 o state to the 7 s 6 d 3 D 1 , 7 s 6 d 3 D 2 , and 7 s 6 d 1 D 2 states and constrain the branching fraction to the 7 s 6 d 3 D 3 state to be less than 0.4% (68% confidence limit). The lifetime of the 3 F 2 o state is determined to be 15 ± 4 ns. Image 1 • Branching ratios out of the 3F 2 o state of radium measured using novel method. • 3F 2 o → 3D 3 branching ratio suppressed by spin-orbit coupling. • Strong 3F 2 o → 1D 2 transition provides spin-flip channel for repumping. • Improved atom slowing using this repumping scheme useful for Schiff EDM search. [ABSTRACT FROM AUTHOR]
Copyright of Spectrochimica Acta Part B is the property of Elsevier B.V. and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
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DbLabel: Engineering Source
An: 146248583
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  Data: Spectroscopic study and lifetime measurement of the 6d7p3F2o state of radium.
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  Data: <searchLink fieldCode="AR" term="%22Booth%2C+D%2EW%2E%22">Booth, D.W.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> dbooth@anl.gov</i><br /><searchLink fieldCode="AR" term="%22Rabga%2C+T%2E%22">Rabga, T.</searchLink><relatesTo>1,2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Ready%2C+R%2E%22">Ready, R.</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Bailey%2C+K%2EG%2E%22">Bailey, K.G.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Bishof%2C+M%2E%22">Bishof, M.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Dietrich%2C+M%2ER%2E%22">Dietrich, M.R.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Greene%2C+J%2EP%2E%22">Greene, J.P.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Mueller%2C+P%2E%22">Mueller, P.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22O'Connor%2C+T%2EP%2E%22">O'Connor, T.P.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Singh%2C+J%2ET%2E%22">Singh, J.T.</searchLink><relatesTo>2</relatesTo> (AUTHOR)
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  Data: <searchLink fieldCode="JN" term="%22Spectrochimica+Acta+Part+B%22">Spectrochimica Acta Part B</searchLink>. Oct2020, Vol. 172, pN.PAG-N.PAG. 1p.
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  Data: <searchLink fieldCode="DE" term="%22Oscillator+strengths%22">Oscillator strengths</searchLink><br /><searchLink fieldCode="DE" term="%22Spin-orbit+interactions%22">Spin-orbit interactions</searchLink><br /><searchLink fieldCode="DE" term="%22Atomic+beams%22">Atomic beams</searchLink><br /><searchLink fieldCode="DE" term="%22Radium%22">Radium</searchLink><br /><searchLink fieldCode="DE" term="%22Branching+ratios%22">Branching ratios</searchLink><br /><searchLink fieldCode="DE" term="%22Metastable+states%22">Metastable states</searchLink>
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  Data: We report a method for the precision measurement of the oscillator strengths and the branching fractions of the decay channels of the 6 d 7 p 3 F 2 o state in 226Ra. This method exploits a set of metastable states present in Ra, allowing a measurement of the oscillator strengths that does not require knowledge of the number of atoms in the atomic beam. We measure the oscillator strengths and the branching fractions for decays from the 6 d 7 p 3 F 2 o state to the 7 s 6 d 3 D 1 , 7 s 6 d 3 D 2 , and 7 s 6 d 1 D 2 states and constrain the branching fraction to the 7 s 6 d 3 D 3 state to be less than 0.4% (68% confidence limit). The lifetime of the 3 F 2 o state is determined to be 15 ± 4 ns. Image 1 • Branching ratios out of the 3F 2 o state of radium measured using novel method. • 3F 2 o → 3D 3 branching ratio suppressed by spin-orbit coupling. • Strong 3F 2 o → 1D 2 transition provides spin-flip channel for repumping. • Improved atom slowing using this repumping scheme useful for Schiff EDM search. [ABSTRACT FROM AUTHOR]
– Name: AbstractSuppliedCopyright
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  Data: <i>Copyright of Spectrochimica Acta Part B is the property of Elsevier B.V. and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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        Value: 10.1016/j.sab.2020.105967
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      – Code: eng
        Text: English
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        StartPage: N.PAG
    Subjects:
      – SubjectFull: Oscillator strengths
        Type: general
      – SubjectFull: Spin-orbit interactions
        Type: general
      – SubjectFull: Atomic beams
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      – SubjectFull: Radium
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      – SubjectFull: Branching ratios
        Type: general
      – SubjectFull: Metastable states
        Type: general
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      – TitleFull: Spectroscopic study and lifetime measurement of the 6d7p3F2o state of radium.
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              Text: Oct2020
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