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Strategic utilization of covalent organic frameworks for uranium adsorption from high concentrate U–Th monazite sand: a review.

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Title: Strategic utilization of covalent organic frameworks for uranium adsorption from high concentrate U–Th monazite sand: a review.
Authors: Saputra, Ade1,2 (AUTHOR) ade.saputra.1@brin.go.id, Abdullah, Iman1 (AUTHOR) iman.abdullah@sci.ui.ac.id, Dahnum, Deliana3 (AUTHOR), Mustika, Deni2 (AUTHOR), Oktavianto, Putra2 (AUTHOR), Noor, Ainun Zakiah4 (AUTHOR), Pamungkas, Niken Siwi2 (AUTHOR), Yusuf, Muhammad5 (AUTHOR) muhammad.yusuf@kfupm.edu.sa
Source: Journal of Radioanalytical & Nuclear Chemistry. Jun2025, Vol. 334 Issue 6, p3843-3864. 22p.
Subjects: Fuel cycle, Bibliometrics, Energy security, Monazite, Tin, Uranium
Abstract: Indonesia's energy independence and net-zero emissions (NZE) goals require sustainable uranium extraction from monazite sand, a tin byproduct. This review evaluates covalent organic frameworks (COFs) for uranium–thorium (U/Th) separation in high-concentration monazite systems. Findings highlight SO3H-functionalized COFs, synthesized via dissolution–precipitation and NH4OH ammonization, as optimal for U/Th separation, exhibiting high uranium adsorption (> 300 mg/g), selectivity, and cost-effectiveness. Their stable porous structures align with Indonesia's monazite processing needs, addressing nuclear fuel cycle challenges. The study underscores COFs' potential to support NZE targets and energy security, urging future research on scalability, regeneration, and industrial integration to transition from lab-scale to practical applications. [ABSTRACT FROM AUTHOR]
Copyright of Journal of Radioanalytical & Nuclear Chemistry is the property of Springer Nature and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
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  Data: Strategic utilization of covalent organic frameworks for uranium adsorption from high concentrate U–Th monazite sand: a review.
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  Data: <searchLink fieldCode="AR" term="%22Saputra%2C+Ade%22">Saputra, Ade</searchLink><relatesTo>1,2</relatesTo> (AUTHOR)<i> ade.saputra.1@brin.go.id</i><br /><searchLink fieldCode="AR" term="%22Abdullah%2C+Iman%22">Abdullah, Iman</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> iman.abdullah@sci.ui.ac.id</i><br /><searchLink fieldCode="AR" term="%22Dahnum%2C+Deliana%22">Dahnum, Deliana</searchLink><relatesTo>3</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Mustika%2C+Deni%22">Mustika, Deni</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Oktavianto%2C+Putra%22">Oktavianto, Putra</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Noor%2C+Ainun+Zakiah%22">Noor, Ainun Zakiah</searchLink><relatesTo>4</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Pamungkas%2C+Niken+Siwi%22">Pamungkas, Niken Siwi</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Yusuf%2C+Muhammad%22">Yusuf, Muhammad</searchLink><relatesTo>5</relatesTo> (AUTHOR)<i> muhammad.yusuf@kfupm.edu.sa</i>
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  Data: <searchLink fieldCode="JN" term="%22Journal+of+Radioanalytical+%26+Nuclear+Chemistry%22">Journal of Radioanalytical & Nuclear Chemistry</searchLink>. Jun2025, Vol. 334 Issue 6, p3843-3864. 22p.
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  Data: <searchLink fieldCode="DE" term="%22Fuel+cycle%22">Fuel cycle</searchLink><br /><searchLink fieldCode="DE" term="%22Bibliometrics%22">Bibliometrics</searchLink><br /><searchLink fieldCode="DE" term="%22Energy+security%22">Energy security</searchLink><br /><searchLink fieldCode="DE" term="%22Monazite%22">Monazite</searchLink><br /><searchLink fieldCode="DE" term="%22Tin%22">Tin</searchLink><br /><searchLink fieldCode="DE" term="%22Uranium%22">Uranium</searchLink>
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  Data: Indonesia's energy independence and net-zero emissions (NZE) goals require sustainable uranium extraction from monazite sand, a tin byproduct. This review evaluates covalent organic frameworks (COFs) for uranium–thorium (U/Th) separation in high-concentration monazite systems. Findings highlight SO3H-functionalized COFs, synthesized via dissolution–precipitation and NH4OH ammonization, as optimal for U/Th separation, exhibiting high uranium adsorption (> 300 mg/g), selectivity, and cost-effectiveness. Their stable porous structures align with Indonesia's monazite processing needs, addressing nuclear fuel cycle challenges. The study underscores COFs' potential to support NZE targets and energy security, urging future research on scalability, regeneration, and industrial integration to transition from lab-scale to practical applications. [ABSTRACT FROM AUTHOR]
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  Label:
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  Data: <i>Copyright of Journal of Radioanalytical & Nuclear Chemistry is the property of Springer Nature and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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        Value: 10.1007/s10967-025-10135-w
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      – Code: eng
        Text: English
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        PageCount: 22
        StartPage: 3843
    Subjects:
      – SubjectFull: Fuel cycle
        Type: general
      – SubjectFull: Bibliometrics
        Type: general
      – SubjectFull: Energy security
        Type: general
      – SubjectFull: Monazite
        Type: general
      – SubjectFull: Tin
        Type: general
      – SubjectFull: Uranium
        Type: general
    Titles:
      – TitleFull: Strategic utilization of covalent organic frameworks for uranium adsorption from high concentrate U–Th monazite sand: a review.
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            NameFull: Saputra, Ade
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            NameFull: Dahnum, Deliana
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            – D: 01
              M: 06
              Text: Jun2025
              Type: published
              Y: 2025
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