Structural, Magnetic and THz Emission Properties of Ultrathin Fe/L1 0 -FePt/Pt Heterostructures.

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Title: Structural, Magnetic and THz Emission Properties of Ultrathin Fe/L1 0 -FePt/Pt Heterostructures.
Authors: Locovei, Claudiu1 (AUTHOR), Torosyan, Garik2 (AUTHOR), Papaioannou, Evangelos Th.1,3 (AUTHOR), Crisan, Alina D.1,4 (AUTHOR), Beigang, Rene1,4 (AUTHOR), Crisan, Ovidiu1,2 (AUTHOR)
Source: Nanomaterials (2079-4991). Jul2025, Vol. 15 Issue 14, p1099. 12p.
Subjects: Heterostructures, Spin Hall effect, Ferromagnetic materials, Submillimeter waves, Platinum alloys, Magnetic coupling, Spintronics
Abstract: Recent achievements in ultrafast spin physics have enabled the use of heterostructures composed of ferromagnetic (FM)/non-magnetic (NM) thin layers for terahertz (THz) generation. The mechanism of THz emission from FM/NM multilayers has been typically ascribed to the inverse spin Hall effect (ISHE). In this work, we probe the mechanism of the ISHE by inserting a second ferromagnetic layer in the form of an alloy between the FM/NM system. In particular, by utilizing the co-sputtering technique, we fabricate Fe/L10-FePt/Pt ultra-thin heterostructures. We successfully grow the tetragonal phase of FePt (L10-phase) as revealed by X-ray diffraction and reflection techniques. We show the strong magnetic coupling between Fe and L10-FePt using magneto-optical and Superconducting Quantum Interference Device (SQUID) magnetometry. Subsequently, by utilizing THz time domain spectroscopy technique, we record the THz emission and thus we the reveal the efficiency of spin-to-charge conversion in Fe/L10-FePt/Pt. We establish that Fe/L10-FePt/Pt configuration is significantly superior to the Fe/Pt bilayer structure, regarding THz emission amplitude. The unique trilayer structure opens new perspectives in terms of material choices for the future spintronic THz sources. [ABSTRACT FROM AUTHOR]
Copyright of Nanomaterials (2079-4991) is the property of MDPI and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
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Items – Name: Title
  Label: Title
  Group: Ti
  Data: Structural, Magnetic and THz Emission Properties of Ultrathin Fe/L1 0 -FePt/Pt Heterostructures.
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  Data: <searchLink fieldCode="AR" term="%22Locovei%2C+Claudiu%22">Locovei, Claudiu</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Torosyan%2C+Garik%22">Torosyan, Garik</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Papaioannou%2C+Evangelos+Th%2E%22">Papaioannou, Evangelos Th.</searchLink><relatesTo>1,3</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Crisan%2C+Alina+D%2E%22">Crisan, Alina D.</searchLink><relatesTo>1,4</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Beigang%2C+Rene%22">Beigang, Rene</searchLink><relatesTo>1,4</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Crisan%2C+Ovidiu%22">Crisan, Ovidiu</searchLink><relatesTo>1,2</relatesTo> (AUTHOR)
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  Data: <searchLink fieldCode="JN" term="%22Nanomaterials+%282079-4991%29%22">Nanomaterials (2079-4991)</searchLink>. Jul2025, Vol. 15 Issue 14, p1099. 12p.
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  Data: <searchLink fieldCode="DE" term="%22Heterostructures%22">Heterostructures</searchLink><br /><searchLink fieldCode="DE" term="%22Spin+Hall+effect%22">Spin Hall effect</searchLink><br /><searchLink fieldCode="DE" term="%22Ferromagnetic+materials%22">Ferromagnetic materials</searchLink><br /><searchLink fieldCode="DE" term="%22Submillimeter+waves%22">Submillimeter waves</searchLink><br /><searchLink fieldCode="DE" term="%22Platinum+alloys%22">Platinum alloys</searchLink><br /><searchLink fieldCode="DE" term="%22Magnetic+coupling%22">Magnetic coupling</searchLink><br /><searchLink fieldCode="DE" term="%22Spintronics%22">Spintronics</searchLink>
– Name: Abstract
  Label: Abstract
  Group: Ab
  Data: Recent achievements in ultrafast spin physics have enabled the use of heterostructures composed of ferromagnetic (FM)/non-magnetic (NM) thin layers for terahertz (THz) generation. The mechanism of THz emission from FM/NM multilayers has been typically ascribed to the inverse spin Hall effect (ISHE). In this work, we probe the mechanism of the ISHE by inserting a second ferromagnetic layer in the form of an alloy between the FM/NM system. In particular, by utilizing the co-sputtering technique, we fabricate Fe/L10-FePt/Pt ultra-thin heterostructures. We successfully grow the tetragonal phase of FePt (L10-phase) as revealed by X-ray diffraction and reflection techniques. We show the strong magnetic coupling between Fe and L10-FePt using magneto-optical and Superconducting Quantum Interference Device (SQUID) magnetometry. Subsequently, by utilizing THz time domain spectroscopy technique, we record the THz emission and thus we the reveal the efficiency of spin-to-charge conversion in Fe/L10-FePt/Pt. We establish that Fe/L10-FePt/Pt configuration is significantly superior to the Fe/Pt bilayer structure, regarding THz emission amplitude. The unique trilayer structure opens new perspectives in terms of material choices for the future spintronic THz sources. [ABSTRACT FROM AUTHOR]
– Name: AbstractSuppliedCopyright
  Label:
  Group: Ab
  Data: <i>Copyright of Nanomaterials (2079-4991) is the property of MDPI and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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      – Type: doi
        Value: 10.3390/nano15141099
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      – Code: eng
        Text: English
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        Type: general
      – SubjectFull: Spin Hall effect
        Type: general
      – SubjectFull: Ferromagnetic materials
        Type: general
      – SubjectFull: Submillimeter waves
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      – SubjectFull: Platinum alloys
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      – SubjectFull: Magnetic coupling
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      – SubjectFull: Spintronics
        Type: general
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      – TitleFull: Structural, Magnetic and THz Emission Properties of Ultrathin Fe/L1 0 -FePt/Pt Heterostructures.
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            NameFull: Locovei, Claudiu
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              M: 07
              Text: Jul2025
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