Polarization spectroscopy of the 5S1/2–5D5/2 two-photon transition in rubidium.

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Title: Polarization spectroscopy of the 5S1/2–5D5/2 two-photon transition in rubidium.
Authors: Busch, H. C.1 (AUTHOR) hauke.busch@gcsu.edu, Busch, C. F.2 (AUTHOR) kwc4mq@virginia.edu, Sukenik, C. I.3 (AUTHOR) csukenik@odu.edu
Source: American Journal of Physics. Oct2025, Vol. 93 Issue 10, p824-834. 11p.
Subjects: Polarization spectroscopy, Rubidium, Atomic transitions, Two-photon absorbing materials, Experimental design, Fluorescence, Atomic physics, Laboratories
Abstract: We describe a one-color, two-photon polarization spectroscopy experiment on the 5S 1 / 2 –5D5/2 transition in rubidium, suitable for implementation in an advanced undergraduate instructional laboratory. The proposed laboratory module synergistically combines polarization spectroscopy with established fluorescence detection at a wavelength different from the excitation wavelength. The curriculum provided in this paper allows students to compare experimental results with predicted theoretical lineshapes and to study the intensity dependence of the two-photon transition. The module also provides a springboard that enables instructors to expand the curriculum to incorporate additional measurements and theoretical analyses. These activities include collecting spectra on additional transitions, measuring the temperature dependence of the spectral amplitudes, or using the dispersive polarization spectra to frequency stabilize a laser without modulation. Editor's Note: This paper describes a polarization spectroscopy experiment in which the 5S–5D transition in rubidium vapor is excited by the absorption of two photons of the same frequency. The authors first provide necessary theoretical background on polarization spectroscopy, then go on to describe their experimental setup. Experimental results are compared with predicted theoretical lineshapes as well as the expected intensity dependence of the two-photon transition. The experiment, which can be performed with a single diode laser, explores topics in atomic physics and optics. It is suitable for the advanced undergraduate instructional laboratory and offers a valuable complement to existing two-photon experiments in rubidium vapor already performed in undergraduate and graduate teaching laboratories. [ABSTRACT FROM AUTHOR]
Copyright of American Journal of Physics is the property of American Institute of Physics and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
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  Data: Polarization spectroscopy of the 5S1/2–5D<subscript>5/2</subscript> two-photon transition in rubidium.
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  Data: <searchLink fieldCode="AR" term="%22Busch%2C+H%2E+C%2E%22">Busch, H. C.</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> hauke.busch@gcsu.edu</i><br /><searchLink fieldCode="AR" term="%22Busch%2C+C%2E+F%2E%22">Busch, C. F.</searchLink><relatesTo>2</relatesTo> (AUTHOR)<i> kwc4mq@virginia.edu</i><br /><searchLink fieldCode="AR" term="%22Sukenik%2C+C%2E+I%2E%22">Sukenik, C. I.</searchLink><relatesTo>3</relatesTo> (AUTHOR)<i> csukenik@odu.edu</i>
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  Data: <searchLink fieldCode="JN" term="%22American+Journal+of+Physics%22">American Journal of Physics</searchLink>. Oct2025, Vol. 93 Issue 10, p824-834. 11p.
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  Data: <searchLink fieldCode="DE" term="%22Polarization+spectroscopy%22">Polarization spectroscopy</searchLink><br /><searchLink fieldCode="DE" term="%22Rubidium%22">Rubidium</searchLink><br /><searchLink fieldCode="DE" term="%22Atomic+transitions%22">Atomic transitions</searchLink><br /><searchLink fieldCode="DE" term="%22Two-photon+absorbing+materials%22">Two-photon absorbing materials</searchLink><br /><searchLink fieldCode="DE" term="%22Experimental+design%22">Experimental design</searchLink><br /><searchLink fieldCode="DE" term="%22Fluorescence%22">Fluorescence</searchLink><br /><searchLink fieldCode="DE" term="%22Atomic+physics%22">Atomic physics</searchLink><br /><searchLink fieldCode="DE" term="%22Laboratories%22">Laboratories</searchLink>
– Name: Abstract
  Label: Abstract
  Group: Ab
  Data: We describe a one-color, two-photon polarization spectroscopy experiment on the 5S 1 / 2 –5D5/2 transition in rubidium, suitable for implementation in an advanced undergraduate instructional laboratory. The proposed laboratory module synergistically combines polarization spectroscopy with established fluorescence detection at a wavelength different from the excitation wavelength. The curriculum provided in this paper allows students to compare experimental results with predicted theoretical lineshapes and to study the intensity dependence of the two-photon transition. The module also provides a springboard that enables instructors to expand the curriculum to incorporate additional measurements and theoretical analyses. These activities include collecting spectra on additional transitions, measuring the temperature dependence of the spectral amplitudes, or using the dispersive polarization spectra to frequency stabilize a laser without modulation. Editor's Note: This paper describes a polarization spectroscopy experiment in which the 5S–5D transition in rubidium vapor is excited by the absorption of two photons of the same frequency. The authors first provide necessary theoretical background on polarization spectroscopy, then go on to describe their experimental setup. Experimental results are compared with predicted theoretical lineshapes as well as the expected intensity dependence of the two-photon transition. The experiment, which can be performed with a single diode laser, explores topics in atomic physics and optics. It is suitable for the advanced undergraduate instructional laboratory and offers a valuable complement to existing two-photon experiments in rubidium vapor already performed in undergraduate and graduate teaching laboratories. [ABSTRACT FROM AUTHOR]
– Name: AbstractSuppliedCopyright
  Label:
  Group: Ab
  Data: <i>Copyright of American Journal of Physics is the property of American Institute of Physics and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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        Value: 10.1119/5.0254590
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        Text: English
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        PageCount: 11
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      – SubjectFull: Polarization spectroscopy
        Type: general
      – SubjectFull: Rubidium
        Type: general
      – SubjectFull: Atomic transitions
        Type: general
      – SubjectFull: Two-photon absorbing materials
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      – SubjectFull: Experimental design
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      – SubjectFull: Fluorescence
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      – SubjectFull: Atomic physics
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      – SubjectFull: Laboratories
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      – TitleFull: Polarization spectroscopy of the 5S1/2–5D5/2 two-photon transition in rubidium.
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              M: 10
              Text: Oct2025
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