Boosting PEM fuel cell cathode performance: The effect of mixing carbon supports on morphology and stability.

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Title: Boosting PEM fuel cell cathode performance: The effect of mixing carbon supports on morphology and stability.
Authors: Laumen, Steffen1,2 (AUTHOR), Burger, Thomas1 (AUTHOR) thomas.burger@freudenberg-eps.com, Bretzler, Patrick1 (AUTHOR), Jurzinsky, Tilman1 (AUTHOR), Ott, Sebastian1 (AUTHOR), Strasser, Peter1,2 (AUTHOR) pstrasser@tu-berlin.de
Source: Journal of Power Sources. Apr2026, Vol. 671, pN.PAG-N.PAG. 1p.
Subjects: Carbon-based materials, Stability (Mechanics), Platinum nanoparticles, Proton exchange membrane fuel cells, Cathode efficiency, Morphology, Durability
Abstract: Carbon catalyst supports significantly impact on the performance and durability of proton exchange membrane fuel cells. Different types of carbon support materials show distinct favorable or detrimental characteristics. In this study, cathodes with platinum nanoparticles deposited on physical mixtures of distinct carbon materials, each with different properties, were prepared, tested, and compared to Pt/C cathodes prepared using each individual carbon support material. The performance of the membrane electrode assemblies (12 cm2 active area) was tested under comparable conditions in single-cell setups using the carbon support accelerated stress test proposed by the U.S. Department of Energy. Physiochemical changes in cathode morphologies and thicknesses were analyzed before and after testing. Our findings demonstrate that by physically combining carbon supports with different properties, a significant increase in morphological stability and layer integrity can be achieved. Moreover, this mixed carbon support approach resulted in a reduction of cathode layer degradation effects such as mass transport limitations and layer collapse during accelerated stress tests. A synergistic effect in the physical mixture of two different carbon types is discussed. We hypothesize that if one type of carbon shows severe degradation under the tested conditions, the other type can compensate and thereby mitigate performance loss. [Display omitted] • Manufacturing fuel cell cathodes with Pt nanoparticles on mixed carbon supports. • Comparative study of activity and durability for Pt/C with single vs mixed supports. • Mixing carbon supports improves cathode durability under stress tests. • Better morphology and porosity retention reduce transport loss and layer collapse. • Synergistic effects of combining different carbon support types. [ABSTRACT FROM AUTHOR]
Copyright of Journal of Power Sources is the property of Elsevier B.V. and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
Database: Engineering Source
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Header DbId: egs
DbLabel: Engineering Source
An: 191760702
AccessLevel: 6
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PubTypeId: academicJournal
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  Label: Title
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  Data: Boosting PEM fuel cell cathode performance: The effect of mixing carbon supports on morphology and stability.
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  Data: <searchLink fieldCode="AR" term="%22Laumen%2C+Steffen%22">Laumen, Steffen</searchLink><relatesTo>1,2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Burger%2C+Thomas%22">Burger, Thomas</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> thomas.burger@freudenberg-eps.com</i><br /><searchLink fieldCode="AR" term="%22Bretzler%2C+Patrick%22">Bretzler, Patrick</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Jurzinsky%2C+Tilman%22">Jurzinsky, Tilman</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Ott%2C+Sebastian%22">Ott, Sebastian</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Strasser%2C+Peter%22">Strasser, Peter</searchLink><relatesTo>1,2</relatesTo> (AUTHOR)<i> pstrasser@tu-berlin.de</i>
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  Data: <searchLink fieldCode="JN" term="%22Journal+of+Power+Sources%22">Journal of Power Sources</searchLink>. Apr2026, Vol. 671, pN.PAG-N.PAG. 1p.
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  Data: <searchLink fieldCode="DE" term="%22Carbon-based+materials%22">Carbon-based materials</searchLink><br /><searchLink fieldCode="DE" term="%22Stability+%28Mechanics%29%22">Stability (Mechanics)</searchLink><br /><searchLink fieldCode="DE" term="%22Platinum+nanoparticles%22">Platinum nanoparticles</searchLink><br /><searchLink fieldCode="DE" term="%22Proton+exchange+membrane+fuel+cells%22">Proton exchange membrane fuel cells</searchLink><br /><searchLink fieldCode="DE" term="%22Cathode+efficiency%22">Cathode efficiency</searchLink><br /><searchLink fieldCode="DE" term="%22Morphology%22">Morphology</searchLink><br /><searchLink fieldCode="DE" term="%22Durability%22">Durability</searchLink>
– Name: Abstract
  Label: Abstract
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  Data: Carbon catalyst supports significantly impact on the performance and durability of proton exchange membrane fuel cells. Different types of carbon support materials show distinct favorable or detrimental characteristics. In this study, cathodes with platinum nanoparticles deposited on physical mixtures of distinct carbon materials, each with different properties, were prepared, tested, and compared to Pt/C cathodes prepared using each individual carbon support material. The performance of the membrane electrode assemblies (12 cm2 active area) was tested under comparable conditions in single-cell setups using the carbon support accelerated stress test proposed by the U.S. Department of Energy. Physiochemical changes in cathode morphologies and thicknesses were analyzed before and after testing. Our findings demonstrate that by physically combining carbon supports with different properties, a significant increase in morphological stability and layer integrity can be achieved. Moreover, this mixed carbon support approach resulted in a reduction of cathode layer degradation effects such as mass transport limitations and layer collapse during accelerated stress tests. A synergistic effect in the physical mixture of two different carbon types is discussed. We hypothesize that if one type of carbon shows severe degradation under the tested conditions, the other type can compensate and thereby mitigate performance loss. [Display omitted] • Manufacturing fuel cell cathodes with Pt nanoparticles on mixed carbon supports. • Comparative study of activity and durability for Pt/C with single vs mixed supports. • Mixing carbon supports improves cathode durability under stress tests. • Better morphology and porosity retention reduce transport loss and layer collapse. • Synergistic effects of combining different carbon support types. [ABSTRACT FROM AUTHOR]
– Name: AbstractSuppliedCopyright
  Label:
  Group: Ab
  Data: <i>Copyright of Journal of Power Sources is the property of Elsevier B.V. and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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RecordInfo BibRecord:
  BibEntity:
    Identifiers:
      – Type: doi
        Value: 10.1016/j.jpowsour.2026.239493
    Languages:
      – Code: eng
        Text: English
    PhysicalDescription:
      Pagination:
        PageCount: 1
        StartPage: N.PAG
    Subjects:
      – SubjectFull: Carbon-based materials
        Type: general
      – SubjectFull: Stability (Mechanics)
        Type: general
      – SubjectFull: Platinum nanoparticles
        Type: general
      – SubjectFull: Proton exchange membrane fuel cells
        Type: general
      – SubjectFull: Cathode efficiency
        Type: general
      – SubjectFull: Morphology
        Type: general
      – SubjectFull: Durability
        Type: general
    Titles:
      – TitleFull: Boosting PEM fuel cell cathode performance: The effect of mixing carbon supports on morphology and stability.
        Type: main
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      – PersonEntity:
          Name:
            NameFull: Laumen, Steffen
      – PersonEntity:
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            NameFull: Burger, Thomas
      – PersonEntity:
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            NameFull: Bretzler, Patrick
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            NameFull: Jurzinsky, Tilman
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            NameFull: Ott, Sebastian
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            NameFull: Strasser, Peter
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          Dates:
            – D: 15
              M: 04
              Text: Apr2026
              Type: published
              Y: 2026
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            – Type: issn-print
              Value: 03787753
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            – Type: volume
              Value: 671
          Titles:
            – TitleFull: Journal of Power Sources
              Type: main
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