Process and Structure Modeling of Architected Thermoplastic Composites Using Shape Forming Elements.

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Title: Process and Structure Modeling of Architected Thermoplastic Composites Using Shape Forming Elements.
Authors: Olanrewaju, Rebecca H.1 (AUTHOR) rebecca_olanrewaju@student.uml.edu, Jiang, Yuefeng2 (AUTHOR), Nguyen, Thao D.1,2 (AUTHOR), Kazmer, David O.1,2 (AUTHOR)
Source: Polymers (20734360). May2026, Vol. 18 Issue 9, p1098. 41p.
Subjects: Polymer liquid crystals, Polyamides, Plastic extrusion, Molecular orientation, Polymeric composites, Mechanical behavior of materials
Abstract: Architected polymer composites use spatially organized phases to achieve targeted property combinations. Shape forming elements (SFEs) are modular coextrusion die inserts that impose internal architectures by reshaping multiple melt streams. This study evaluates three SFE designs (Jacks, I-Beam, and Barn Door) that position a liquid crystalline polymer (LCP) and an amorphous polyamide (APA) in distinct core–shell configurations. Polymer clay prototyping and ANSYS Polyflow simulations were used to screen flow behavior, followed by extrusion at two puller speeds and characterization via optical microscopy and tensile testing. Microscopy revealed that abrupt area transitions and viscosity contrast disrupt encapsulation and distort designed features. Regression analysis showed that LCP content governs stiffness and strength, while higher puller speed enhances reinforcement through molecular orientation. Cross sectional geometries were quantified using interfacial perimeter, moments of inertia, and polar dispersion ratios, and correlated to tensile performance. Increased interfacial length reduced modulus, strength, and ductility. Modulus improved with LCP orientation and confinement, strength increased when LCP was placed at vertical extremities, and elongation was maximized by horizontally distributing LCP within a thick APA shell. These results demonstrate that SFEs enable tunable tradeoffs between stiffness, strength, and ductility. [ABSTRACT FROM AUTHOR]
Copyright of Polymers (20734360) is the property of MDPI and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
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  Data: Process and Structure Modeling of Architected Thermoplastic Composites Using Shape Forming Elements.
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  Data: <searchLink fieldCode="JN" term="%22Polymers+%2820734360%29%22">Polymers (20734360)</searchLink>. May2026, Vol. 18 Issue 9, p1098. 41p.
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  Data: <searchLink fieldCode="DE" term="%22Polymer+liquid+crystals%22">Polymer liquid crystals</searchLink><br /><searchLink fieldCode="DE" term="%22Polyamides%22">Polyamides</searchLink><br /><searchLink fieldCode="DE" term="%22Plastic+extrusion%22">Plastic extrusion</searchLink><br /><searchLink fieldCode="DE" term="%22Molecular+orientation%22">Molecular orientation</searchLink><br /><searchLink fieldCode="DE" term="%22Polymeric+composites%22">Polymeric composites</searchLink><br /><searchLink fieldCode="DE" term="%22Mechanical+behavior+of+materials%22">Mechanical behavior of materials</searchLink>
– Name: Abstract
  Label: Abstract
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  Data: Architected polymer composites use spatially organized phases to achieve targeted property combinations. Shape forming elements (SFEs) are modular coextrusion die inserts that impose internal architectures by reshaping multiple melt streams. This study evaluates three SFE designs (Jacks, I-Beam, and Barn Door) that position a liquid crystalline polymer (LCP) and an amorphous polyamide (APA) in distinct core–shell configurations. Polymer clay prototyping and ANSYS Polyflow simulations were used to screen flow behavior, followed by extrusion at two puller speeds and characterization via optical microscopy and tensile testing. Microscopy revealed that abrupt area transitions and viscosity contrast disrupt encapsulation and distort designed features. Regression analysis showed that LCP content governs stiffness and strength, while higher puller speed enhances reinforcement through molecular orientation. Cross sectional geometries were quantified using interfacial perimeter, moments of inertia, and polar dispersion ratios, and correlated to tensile performance. Increased interfacial length reduced modulus, strength, and ductility. Modulus improved with LCP orientation and confinement, strength increased when LCP was placed at vertical extremities, and elongation was maximized by horizontally distributing LCP within a thick APA shell. These results demonstrate that SFEs enable tunable tradeoffs between stiffness, strength, and ductility. [ABSTRACT FROM AUTHOR]
– Name: AbstractSuppliedCopyright
  Label:
  Group: Ab
  Data: <i>Copyright of Polymers (20734360) is the property of MDPI and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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RecordInfo BibRecord:
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      – Type: doi
        Value: 10.3390/polym18091098
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      – Code: eng
        Text: English
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        PageCount: 41
        StartPage: 1098
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      – SubjectFull: Polymer liquid crystals
        Type: general
      – SubjectFull: Polyamides
        Type: general
      – SubjectFull: Plastic extrusion
        Type: general
      – SubjectFull: Molecular orientation
        Type: general
      – SubjectFull: Polymeric composites
        Type: general
      – SubjectFull: Mechanical behavior of materials
        Type: general
    Titles:
      – TitleFull: Process and Structure Modeling of Architected Thermoplastic Composites Using Shape Forming Elements.
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            NameFull: Olanrewaju, Rebecca H.
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            NameFull: Jiang, Yuefeng
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            NameFull: Nguyen, Thao D.
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            NameFull: Kazmer, David O.
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            – D: 01
              M: 05
              Text: May2026
              Type: published
              Y: 2026
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