Effects of Core–Shell Heterogeneous Grain Structure Topology on Tensile Strength of CoCrFeMnNi High-Entropy Alloy Based on Crystal Plasticity Modeling.

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Title: Effects of Core–Shell Heterogeneous Grain Structure Topology on Tensile Strength of CoCrFeMnNi High-Entropy Alloy Based on Crystal Plasticity Modeling.
Authors: Fu, Rubing1 (AUTHOR), Wang, Xin2 (AUTHOR), Zhang, Zhe1 (AUTHOR) zhe.zhang@tju.edu.cn, Chen, Gang1,2 (AUTHOR)
Source: Materials (1996-1944). Jun2026, Vol. 19 Issue 12, p2433. 27p.
Subjects: Tensile strength, Microstructure, Grain size, High-entropy alloys, Strain hardening, Material plasticity
Abstract: Heterogeneous grain structured design has emerged as an effective strategy to overcome the limitations of mechanical properties in structural materials. Core–shell heterogeneous grain structured materials exhibit a good strength-ductility synergy owing to their continuously networked grain topology. However, controlling the grain size and fraction in core–shell structures through mechanical milling and powder metallurgy remains challenging. Therefore, the effects of grain structure topology on mechanical behavior remain unclear. This study establishes a crystal plastic finite element (CPFE) model of a core–shell structure and discusses the effects of core–shell topological characteristics, i.e., core–shell fraction (Sf = 15% to 65%), the core–shell interface gradient (θ = 63° to 90°), and the coarse grain/ultrafine grain size ratio (CG/UFG = 8/2 to 8/1), on tensile strength and hetero-deformation induced (HDI) hardening. The results indicate that the tensile strength is strongly correlated with the core–shell fraction and CG/UFG size ratio. The tensile strength is enhanced with increasing core–shell fraction and CG/UFG size ratio, which can be attributed to the increased fraction of ultrafine grains and their reduced grain size. The tensile strength increases by approximately 30% when the core–shell fraction increases from 15% to 65%, and increases by approximately 12% when the CG/UFG size ratio changes from 8/2 to 8/1. However, these two parameters exhibit a negligible influence on HDI hardening. In contrast, compared to θ = 63°, the HDI hardening at θ = 90° increases by approximately 20%, thus it indicates the sharp core–shell interface gradient markedly promotes HDI hardening, thereby improving the tensile strength through an increased hardening rate. Collectively, this study provides useful information for the microstructure design of core–shell heterogeneous grain structured materials. [ABSTRACT FROM AUTHOR]
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  Data: Effects of Core–Shell Heterogeneous Grain Structure Topology on Tensile Strength of CoCrFeMnNi High-Entropy Alloy Based on Crystal Plasticity Modeling.
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  Data: <searchLink fieldCode="AR" term="%22Fu%2C+Rubing%22">Fu, Rubing</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Wang%2C+Xin%22">Wang, Xin</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Zhang%2C+Zhe%22">Zhang, Zhe</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> zhe.zhang@tju.edu.cn</i><br /><searchLink fieldCode="AR" term="%22Chen%2C+Gang%22">Chen, Gang</searchLink><relatesTo>1,2</relatesTo> (AUTHOR)
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  Data: <searchLink fieldCode="JN" term="%22Materials+%281996-1944%29%22">Materials (1996-1944)</searchLink>. Jun2026, Vol. 19 Issue 12, p2433. 27p.
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  Data: <searchLink fieldCode="DE" term="%22Tensile+strength%22">Tensile strength</searchLink><br /><searchLink fieldCode="DE" term="%22Microstructure%22">Microstructure</searchLink><br /><searchLink fieldCode="DE" term="%22Grain+size%22">Grain size</searchLink><br /><searchLink fieldCode="DE" term="%22High-entropy+alloys%22">High-entropy alloys</searchLink><br /><searchLink fieldCode="DE" term="%22Strain+hardening%22">Strain hardening</searchLink><br /><searchLink fieldCode="DE" term="%22Material+plasticity%22">Material plasticity</searchLink>
– Name: Abstract
  Label: Abstract
  Group: Ab
  Data: Heterogeneous grain structured design has emerged as an effective strategy to overcome the limitations of mechanical properties in structural materials. Core–shell heterogeneous grain structured materials exhibit a good strength-ductility synergy owing to their continuously networked grain topology. However, controlling the grain size and fraction in core–shell structures through mechanical milling and powder metallurgy remains challenging. Therefore, the effects of grain structure topology on mechanical behavior remain unclear. This study establishes a crystal plastic finite element (CPFE) model of a core–shell structure and discusses the effects of core–shell topological characteristics, i.e., core–shell fraction (Sf = 15% to 65%), the core–shell interface gradient (θ = 63° to 90°), and the coarse grain/ultrafine grain size ratio (CG/UFG = 8/2 to 8/1), on tensile strength and hetero-deformation induced (HDI) hardening. The results indicate that the tensile strength is strongly correlated with the core–shell fraction and CG/UFG size ratio. The tensile strength is enhanced with increasing core–shell fraction and CG/UFG size ratio, which can be attributed to the increased fraction of ultrafine grains and their reduced grain size. The tensile strength increases by approximately 30% when the core–shell fraction increases from 15% to 65%, and increases by approximately 12% when the CG/UFG size ratio changes from 8/2 to 8/1. However, these two parameters exhibit a negligible influence on HDI hardening. In contrast, compared to θ = 63°, the HDI hardening at θ = 90° increases by approximately 20%, thus it indicates the sharp core–shell interface gradient markedly promotes HDI hardening, thereby improving the tensile strength through an increased hardening rate. Collectively, this study provides useful information for the microstructure design of core–shell heterogeneous grain structured materials. [ABSTRACT FROM AUTHOR]
– Name: AbstractSuppliedCopyright
  Label:
  Group: Ab
  Data: <i>Copyright of Materials (1996-1944) is the property of MDPI and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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        Value: 10.3390/ma19122433
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      – Code: eng
        Text: English
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        PageCount: 27
        StartPage: 2433
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      – SubjectFull: Tensile strength
        Type: general
      – SubjectFull: Microstructure
        Type: general
      – SubjectFull: Grain size
        Type: general
      – SubjectFull: High-entropy alloys
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      – SubjectFull: Strain hardening
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      – SubjectFull: Material plasticity
        Type: general
    Titles:
      – TitleFull: Effects of Core–Shell Heterogeneous Grain Structure Topology on Tensile Strength of CoCrFeMnNi High-Entropy Alloy Based on Crystal Plasticity Modeling.
        Type: main
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            NameFull: Fu, Rubing
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            NameFull: Wang, Xin
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            NameFull: Zhang, Zhe
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            NameFull: Chen, Gang
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            – D: 15
              M: 06
              Text: Jun2026
              Type: published
              Y: 2026
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              Value: 19
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