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Preparation of methylammonium lead iodide (CH3NH3PbI3) thin film perovskite solar cells by chemical vapor deposition using methylamine gas (CH3NH2) and hydrogen iodide gas.

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Title: Preparation of methylammonium lead iodide (CH3NH3PbI3) thin film perovskite solar cells by chemical vapor deposition using methylamine gas (CH3NH2) and hydrogen iodide gas.
Authors: Mortan, Claudiu1 (AUTHOR) cmortan@surface.tu-darmstadt.de, Hellmann, Tim1 (AUTHOR), Buchhorn, Moritz1 (AUTHOR), d'Eril Melzi, Marco1 (AUTHOR), Clemens, Oliver2 (AUTHOR), Mayer, Thomas1 (AUTHOR), Jaegermann, Wolfram1 (AUTHOR)
Source: Energy Science & Engineering. Sep2020, Vol. 8 Issue 9, p3165-3173. 9p.
Subject Terms: *Chemical vapor deposition, *Perovskite, *Solar cells, *Lead iodide, *Thin films, *Lead oxides, *Dye-sensitized solar cells
Abstract: An upscalable chemical vapor deposition setup has been built‐up and employed in producing methylammonium lead iodide (MAPI) thin film perovskite solar cells, leading to a maximum efficiency of 12.9%. The method makes use of methylamine gas and hydrogen iodide gas to transform a predeposited layer of lead(II)iodide (PbI2) into MAPI. Although the reaction mechanism includes the intermediate phases lead oxide (PbO) and lead hydroxide (Pb(OH)2), indicated at least on the surface of the samples by XPS, neither species could be observed in XRD measurements of the stepwise reaction, which show a mixture of highly oriented cubic and tetragonal MAPI perovskite lattice systems. [ABSTRACT FROM AUTHOR]
Database: Energy & Power Source
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An: 145429904
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  Label: Title
  Group: Ti
  Data: Preparation of methylammonium lead iodide (CH<subscript>3</subscript>NH<subscript>3</subscript>PbI<subscript>3</subscript>) thin film perovskite solar cells by chemical vapor deposition using methylamine gas (CH<subscript>3</subscript>NH<subscript>2</subscript>) and hydrogen iodide gas.
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  Data: <searchLink fieldCode="AR" term="%22Mortan%2C+Claudiu%22">Mortan, Claudiu</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> cmortan@surface.tu-darmstadt.de</i><br /><searchLink fieldCode="AR" term="%22Hellmann%2C+Tim%22">Hellmann, Tim</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Buchhorn%2C+Moritz%22">Buchhorn, Moritz</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22d'Eril+Melzi%2C+Marco%22">d'Eril Melzi, Marco</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Clemens%2C+Oliver%22">Clemens, Oliver</searchLink><relatesTo>2</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Mayer%2C+Thomas%22">Mayer, Thomas</searchLink><relatesTo>1</relatesTo> (AUTHOR)<br /><searchLink fieldCode="AR" term="%22Jaegermann%2C+Wolfram%22">Jaegermann, Wolfram</searchLink><relatesTo>1</relatesTo> (AUTHOR)
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  Data: <searchLink fieldCode="JN" term="%22Energy+Science+%26+Engineering%22">Energy Science & Engineering</searchLink>. Sep2020, Vol. 8 Issue 9, p3165-3173. 9p.
– Name: Subject
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  Data: *<searchLink fieldCode="DE" term="%22Chemical+vapor+deposition%22">Chemical vapor deposition</searchLink><br />*<searchLink fieldCode="DE" term="%22Perovskite%22">Perovskite</searchLink><br />*<searchLink fieldCode="DE" term="%22Solar+cells%22">Solar cells</searchLink><br />*<searchLink fieldCode="DE" term="%22Lead+iodide%22">Lead iodide</searchLink><br />*<searchLink fieldCode="DE" term="%22Thin+films%22">Thin films</searchLink><br />*<searchLink fieldCode="DE" term="%22Lead+oxides%22">Lead oxides</searchLink><br />*<searchLink fieldCode="DE" term="%22Dye-sensitized+solar+cells%22">Dye-sensitized solar cells</searchLink>
– Name: Abstract
  Label: Abstract
  Group: Ab
  Data: An upscalable chemical vapor deposition setup has been built‐up and employed in producing methylammonium lead iodide (MAPI) thin film perovskite solar cells, leading to a maximum efficiency of 12.9%. The method makes use of methylamine gas and hydrogen iodide gas to transform a predeposited layer of lead(II)iodide (PbI2) into MAPI. Although the reaction mechanism includes the intermediate phases lead oxide (PbO) and lead hydroxide (Pb(OH)2), indicated at least on the surface of the samples by XPS, neither species could be observed in XRD measurements of the stepwise reaction, which show a mixture of highly oriented cubic and tetragonal MAPI perovskite lattice systems. [ABSTRACT FROM AUTHOR]
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RecordInfo BibRecord:
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    Identifiers:
      – Type: doi
        Value: 10.1002/ese3.734
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      – Code: eng
        Text: English
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        PageCount: 9
        StartPage: 3165
    Subjects:
      – SubjectFull: Chemical vapor deposition
        Type: general
      – SubjectFull: Perovskite
        Type: general
      – SubjectFull: Solar cells
        Type: general
      – SubjectFull: Lead iodide
        Type: general
      – SubjectFull: Thin films
        Type: general
      – SubjectFull: Lead oxides
        Type: general
      – SubjectFull: Dye-sensitized solar cells
        Type: general
    Titles:
      – TitleFull: Preparation of methylammonium lead iodide (CH3NH3PbI3) thin film perovskite solar cells by chemical vapor deposition using methylamine gas (CH3NH2) and hydrogen iodide gas.
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          Name:
            NameFull: Mortan, Claudiu
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            NameFull: Hellmann, Tim
      – PersonEntity:
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            NameFull: Buchhorn, Moritz
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            NameFull: d'Eril Melzi, Marco
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            NameFull: Clemens, Oliver
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            NameFull: Mayer, Thomas
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            NameFull: Jaegermann, Wolfram
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            – D: 01
              M: 09
              Text: Sep2020
              Type: published
              Y: 2020
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              Value: 20500505
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              Value: 8
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              Value: 9
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            – TitleFull: Energy Science & Engineering
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