Evaluation of MERRA-2 PM2.5 species at three locations in India and their historical (1999–2019) trends.
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| Title: | Evaluation of MERRA-2 PM |
|---|---|
| Authors: | Devaliya, Sandeep1 (AUTHOR) sandeep.nitb92@gmail.com, Patra, Sayak1 (AUTHOR) sayak23@iiserb.ac.in, Maheshwarkar, Prem1 (AUTHOR) prem.97mah.pm@gmail.com, Bhardwaj, Ankur1 (AUTHOR) ankurbhardwaj567@gmail.com, Haswani, Diksha1 (AUTHOR) haswani19@iiserb.ac.in, Shukla, Deeksha1 (AUTHOR) deeksha19.iiserb@gmail.com, Sunder Raman, Ramya1 (AUTHOR) ramyasr@iiserb.ac.in, Dhandapani, Abisheg2 (AUTHOR) abishegdhandapani@gmail.com, Kumar, R. Naresh2 (AUTHOR) rnaresh@bitmesra.ac.in, K. P., Jithin3 (AUTHOR) kp.jithin@gmail.com, Kaggere, Lokesh3 (AUTHOR) lokesh.kaggere@gmail.com |
| Source: | Environmental Monitoring & Assessment. May2026, Vol. 198 Issue 5, p1-19. 19p. |
| Subject Terms: | *Chemical speciation, *Trend analysis, *Atmospheric aerosols, *Particulate matter, *Air quality monitoring, *Aerosols, *Retrospective studies, *Climate change |
| Geographic Terms: | India, Mysuru (India) |
| Abstract: | Surface PM2.5 mass reconstructed from MERRA-2 (Modern Era-Retrospective analysis for Research and Applications) chemical species is widely used to assess aerosol-climate interactions and human health impacts, globally. However, species-wise validation of MERRA-2 PM2.5 against in-situ measurements remains sparse over India due to limited ground-based aerosol speciation data. This study presents the first species-wise validation of MERRA-2 PM2.5 components (organic carbon (OC), black carbon (BC), sulfate, sea-salt, and dust) using year-long (2019) in-situ measurements of PM2.5 and its chemical constituents at three geographically distinct Indian sites—Bhopal (central India), Mesra (eastern India), and Mysuru (southern India). Across the study sites, with reference to in-situ species, MERRA-2 OC showed variable agreement, ranging from underestimation (− 23%) to overestimation (+ 22%), while sulfate was predominantly underestimated (− 31% to − 0.36%). Dust and sea-salt were consistently overestimated (+ 36% to + 65% and + 33% to + 300%, respectively), with poor sea-salt correlations (correlation coefficient < 0.2). The annual mean reconstructed MERRA-2 PM2.5 mass (excluding nitrate) underestimated in-situ PM2.5 by 9–27%. Incorporation of estimated nitrate, derived from nitrate-to-sulfate ratios from the CAMS (Copernicus Atmosphere Monitoring Service) reanalysis, reduced the underestimation to 9–17% at Mesra and Mysuru, and resulted in a slight overestimation (2%) at Bhopal. Mann-Kendall trend analysis (1999–2019) of the MERRA-2 species revealed increasing anthropogenic aerosol species (sulfate, OC, and BC), particularly over eastern and central India, likely driven by coal-based power generation and residential biomass burning. These validated, species-wise MERRA-2 PM2.5 products provide a robust supplementary resource for aerosol, air-quality, climate, and health assessments across India. [ABSTRACT FROM AUTHOR] |
| Database: | Energy & Power Source |
| FullText | Text: Availability: 0 |
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| Header | DbId: enr DbLabel: Energy & Power Source An: 193884609 AccessLevel: 6 PubType: Academic Journal PubTypeId: academicJournal PreciseRelevancyScore: 0 |
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| Items | – Name: Title Label: Title Group: Ti Data: Evaluation of MERRA-2 PM<subscript>2.5</subscript> species at three locations in India and their historical (1999–2019) trends. – Name: Author Label: Authors Group: Au Data: <searchLink fieldCode="AR" term="%22Devaliya%2C+Sandeep%22">Devaliya, Sandeep</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> sandeep.nitb92@gmail.com</i><br /><searchLink fieldCode="AR" term="%22Patra%2C+Sayak%22">Patra, Sayak</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> sayak23@iiserb.ac.in</i><br /><searchLink fieldCode="AR" term="%22Maheshwarkar%2C+Prem%22">Maheshwarkar, Prem</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> prem.97mah.pm@gmail.com</i><br /><searchLink fieldCode="AR" term="%22Bhardwaj%2C+Ankur%22">Bhardwaj, Ankur</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> ankurbhardwaj567@gmail.com</i><br /><searchLink fieldCode="AR" term="%22Haswani%2C+Diksha%22">Haswani, Diksha</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> haswani19@iiserb.ac.in</i><br /><searchLink fieldCode="AR" term="%22Shukla%2C+Deeksha%22">Shukla, Deeksha</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> deeksha19.iiserb@gmail.com</i><br /><searchLink fieldCode="AR" term="%22Sunder+Raman%2C+Ramya%22">Sunder Raman, Ramya</searchLink><relatesTo>1</relatesTo> (AUTHOR)<i> ramyasr@iiserb.ac.in</i><br /><searchLink fieldCode="AR" term="%22Dhandapani%2C+Abisheg%22">Dhandapani, Abisheg</searchLink><relatesTo>2</relatesTo> (AUTHOR)<i> abishegdhandapani@gmail.com</i><br /><searchLink fieldCode="AR" term="%22Kumar%2C+R%2E+Naresh%22">Kumar, R. Naresh</searchLink><relatesTo>2</relatesTo> (AUTHOR)<i> rnaresh@bitmesra.ac.in</i><br /><searchLink fieldCode="AR" term="%22K%2E+P%2E%2C+Jithin%22">K. P., Jithin</searchLink><relatesTo>3</relatesTo> (AUTHOR)<i> kp.jithin@gmail.com</i><br /><searchLink fieldCode="AR" term="%22Kaggere%2C+Lokesh%22">Kaggere, Lokesh</searchLink><relatesTo>3</relatesTo> (AUTHOR)<i> lokesh.kaggere@gmail.com</i> – Name: TitleSource Label: Source Group: Src Data: <searchLink fieldCode="JN" term="%22Environmental+Monitoring+%26+Assessment%22">Environmental Monitoring & Assessment</searchLink>. May2026, Vol. 198 Issue 5, p1-19. 19p. – Name: Subject Label: Subject Terms Group: Su Data: *<searchLink fieldCode="DE" term="%22Chemical+speciation%22">Chemical speciation</searchLink><br />*<searchLink fieldCode="DE" term="%22Trend+analysis%22">Trend analysis</searchLink><br />*<searchLink fieldCode="DE" term="%22Atmospheric+aerosols%22">Atmospheric aerosols</searchLink><br />*<searchLink fieldCode="DE" term="%22Particulate+matter%22">Particulate matter</searchLink><br />*<searchLink fieldCode="DE" term="%22Air+quality+monitoring%22">Air quality monitoring</searchLink><br />*<searchLink fieldCode="DE" term="%22Aerosols%22">Aerosols</searchLink><br />*<searchLink fieldCode="DE" term="%22Retrospective+studies%22">Retrospective studies</searchLink><br />*<searchLink fieldCode="DE" term="%22Climate+change%22">Climate change</searchLink> – Name: SubjectGeographic Label: Geographic Terms Group: Su Data: <searchLink fieldCode="DE" term="%22India%22">India</searchLink><br /><searchLink fieldCode="DE" term="%22Mysuru+%28India%29%22">Mysuru (India)</searchLink> – Name: Abstract Label: Abstract Group: Ab Data: Surface PM2.5 mass reconstructed from MERRA-2 (Modern Era-Retrospective analysis for Research and Applications) chemical species is widely used to assess aerosol-climate interactions and human health impacts, globally. However, species-wise validation of MERRA-2 PM2.5 against in-situ measurements remains sparse over India due to limited ground-based aerosol speciation data. This study presents the first species-wise validation of MERRA-2 PM2.5 components (organic carbon (OC), black carbon (BC), sulfate, sea-salt, and dust) using year-long (2019) in-situ measurements of PM2.5 and its chemical constituents at three geographically distinct Indian sites—Bhopal (central India), Mesra (eastern India), and Mysuru (southern India). Across the study sites, with reference to in-situ species, MERRA-2 OC showed variable agreement, ranging from underestimation (− 23%) to overestimation (+ 22%), while sulfate was predominantly underestimated (− 31% to − 0.36%). Dust and sea-salt were consistently overestimated (+ 36% to + 65% and + 33% to + 300%, respectively), with poor sea-salt correlations (correlation coefficient < 0.2). The annual mean reconstructed MERRA-2 PM2.5 mass (excluding nitrate) underestimated in-situ PM2.5 by 9–27%. Incorporation of estimated nitrate, derived from nitrate-to-sulfate ratios from the CAMS (Copernicus Atmosphere Monitoring Service) reanalysis, reduced the underestimation to 9–17% at Mesra and Mysuru, and resulted in a slight overestimation (2%) at Bhopal. Mann-Kendall trend analysis (1999–2019) of the MERRA-2 species revealed increasing anthropogenic aerosol species (sulfate, OC, and BC), particularly over eastern and central India, likely driven by coal-based power generation and residential biomass burning. These validated, species-wise MERRA-2 PM2.5 products provide a robust supplementary resource for aerosol, air-quality, climate, and health assessments across India. [ABSTRACT FROM AUTHOR] |
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| RecordInfo | BibRecord: BibEntity: Identifiers: – Type: doi Value: 10.1007/s10661-026-15175-7 Languages: – Code: eng Text: English PhysicalDescription: Pagination: PageCount: 19 StartPage: 1 Subjects: – SubjectFull: Chemical speciation Type: general – SubjectFull: Trend analysis Type: general – SubjectFull: Atmospheric aerosols Type: general – SubjectFull: Particulate matter Type: general – SubjectFull: Air quality monitoring Type: general – SubjectFull: Aerosols Type: general – SubjectFull: Retrospective studies Type: general – SubjectFull: Climate change Type: general – SubjectFull: India Type: general – SubjectFull: Mysuru (India) Type: general Titles: – TitleFull: Evaluation of MERRA-2 PM2.5 species at three locations in India and their historical (1999–2019) trends. Type: main BibRelationships: HasContributorRelationships: – PersonEntity: Name: NameFull: Devaliya, Sandeep – PersonEntity: Name: NameFull: Patra, Sayak – PersonEntity: Name: NameFull: Maheshwarkar, Prem – PersonEntity: Name: NameFull: Bhardwaj, Ankur – PersonEntity: Name: NameFull: Haswani, Diksha – PersonEntity: Name: NameFull: Shukla, Deeksha – PersonEntity: Name: NameFull: Sunder Raman, Ramya – PersonEntity: Name: NameFull: Dhandapani, Abisheg – PersonEntity: Name: NameFull: Kumar, R. Naresh – PersonEntity: Name: NameFull: K. P., Jithin – PersonEntity: Name: NameFull: Kaggere, Lokesh IsPartOfRelationships: – BibEntity: Dates: – D: 01 M: 05 Text: May2026 Type: published Y: 2026 Identifiers: – Type: issn-print Value: 01676369 Numbering: – Type: volume Value: 198 – Type: issue Value: 5 Titles: – TitleFull: Environmental Monitoring & Assessment Type: main |
| ResultId | 1 |