Squeezed dual-comb spectroscopy.

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Bibliographic Details
Title: Squeezed dual-comb spectroscopy.
Authors: Herman, Daniel I. (AUTHOR), Walsh, Mathieu (AUTHOR), Kreider, Molly Kate (AUTHOR), Lordi, Noah (AUTHOR), Tsao, Eugene J. (AUTHOR), Lind, Alexander J. (AUTHOR), Heyrich, Matthew (AUTHOR), Combes, Joshua (AUTHOR), Genest, Jérôme (AUTHOR), Diddams, Scott A. (AUTHOR)
Source: Science (pre-March 2025). 2/7/2025, Vol. 387 Issue 6734, p653-658. 6p. 7 Color Photographs.
Subjects: Kerr electro-optical effect, Continuous wave lasers, Frequency combs, Quantum noise, Quantum mechanics, Squeezed light
Abstract: Optical frequency combs have enabled distinct advantages in broadband, high-resolution spectroscopy and precision interferometry. However, quantum mechanics ultimately limits the metrological precision achievable with laser frequency combs. Quantum squeezing has led to substantial measurement improvements with continuous wave lasers, but experiments demonstrating metrological advantage with squeezed combs are less developed. Using the Kerr effect in nonlinear optical fiber, a 1-gigahertz frequency comb centered at 1560 nanometers is amplitude-squeezed by >3 decibels (dB) over a 2.5-terahertz bandwidth. Dual-comb interferometry yields mode-resolved spectroscopy of hydrogen sulfide gas with a signal-to-noise ratio nearly 3 dB beyond the shot-noise limit. The quantum noise reduction leads to a twofold quantum speedup in the determination of gas concentration, with implications for high-speed measurements of multiple species in dynamic chemical environments. [ABSTRACT FROM AUTHOR]
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Database: Psychology and Behavioral Sciences Collection
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Abstract:Optical frequency combs have enabled distinct advantages in broadband, high-resolution spectroscopy and precision interferometry. However, quantum mechanics ultimately limits the metrological precision achievable with laser frequency combs. Quantum squeezing has led to substantial measurement improvements with continuous wave lasers, but experiments demonstrating metrological advantage with squeezed combs are less developed. Using the Kerr effect in nonlinear optical fiber, a 1-gigahertz frequency comb centered at 1560 nanometers is amplitude-squeezed by >3 decibels (dB) over a 2.5-terahertz bandwidth. Dual-comb interferometry yields mode-resolved spectroscopy of hydrogen sulfide gas with a signal-to-noise ratio nearly 3 dB beyond the shot-noise limit. The quantum noise reduction leads to a twofold quantum speedup in the determination of gas concentration, with implications for high-speed measurements of multiple species in dynamic chemical environments. [ABSTRACT FROM AUTHOR]
ISSN:00368075
DOI:10.1126/science.ads6292