Biocatalytic methanation of hydrogen and carbon dioxide in an anaerobic three-phase system.

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Bibliographic Details
Title: Biocatalytic methanation of hydrogen and carbon dioxide in an anaerobic three-phase system.
Authors: Burkhardt, M.1 Burkhardt@tu-cottbus.de, Koschack, T.1, Busch, G.1
Source: Bioresource Technology. Feb2015, Vol. 178, p330-333. 4p.
Subjects: Biocatalysis, Methanation, Hydrogen, Carbon dioxide, Anaerobic digestion, Trickle bed reactors
Abstract: A new type of anaerobic trickle-bed reactor was used for biocatalytic methanation of hydrogen and carbon dioxide under mesophilic temperatures and ambient pressure in a continuous process. The conversion of gaseous substrates through immobilized hydrogenotrophic methanogenic archaea in a biofilm is a unique feature of this type of reactor. Due to the formation of a three-phase system on the carrier surface and operation as a plug flow reactor without gas recirculation, a complete reaction could be observed. With a methane concentration higher than c CH 4 = 98 % , the product gas exhibits a very high quality. A specific methane production of P CH 4 = 1.49 Nm 3 / ( m SV 3 d ) was achieved at a hydraulic loading rate of LR H 2 = 6.0 Nm 3 / ( m SV 3 d ) . The relation between trickle flow through the reactor and productivity could be shown. An application for methane enrichment in combination with biogas facilities as a source of carbon dioxide has also been positively proven. [ABSTRACT FROM AUTHOR]
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Database: Engineering Source
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Abstract:A new type of anaerobic trickle-bed reactor was used for biocatalytic methanation of hydrogen and carbon dioxide under mesophilic temperatures and ambient pressure in a continuous process. The conversion of gaseous substrates through immobilized hydrogenotrophic methanogenic archaea in a biofilm is a unique feature of this type of reactor. Due to the formation of a three-phase system on the carrier surface and operation as a plug flow reactor without gas recirculation, a complete reaction could be observed. With a methane concentration higher than c CH 4 = 98 % , the product gas exhibits a very high quality. A specific methane production of P CH 4 = 1.49 Nm 3 / ( m SV 3 d ) was achieved at a hydraulic loading rate of LR H 2 = 6.0 Nm 3 / ( m SV 3 d ) . The relation between trickle flow through the reactor and productivity could be shown. An application for methane enrichment in combination with biogas facilities as a source of carbon dioxide has also been positively proven. [ABSTRACT FROM AUTHOR]
ISSN:09608524
DOI:10.1016/j.biortech.2014.08.023