Laser-induced forward transfer of high viscosity graphene inks.
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| Title: | Laser-induced forward transfer of high viscosity graphene inks. |
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| Authors: | Dilmy, Dawood1,2 (AUTHOR) ddd179@student.bham.ac.uk, Gaddam, Anvesh1 (AUTHOR), Cummins, Gerard1 (AUTHOR), Dimov, Stefan1 (AUTHOR) |
| Source: | Applied Physics A: Materials Science & Processing. Apr2025, Vol. 131 Issue 4, p1-16. 16p. |
| Subjects: | Conductive ink, Printed electronics, Electric circuits, Phenomenology, Printed circuits |
| Abstract: | Laser-induced forward transfer (LIFT) is gaining significant attention as a non-contact printing technique for high-viscosity conductive inks in printed electronics. However, the high wet thickness of printed tracks is essential for achieving effective electrical pathways, a requirement that has not been thoroughly considered so far. The wet thickness is a function of ink viscosity, substrate wettability, and the laser processing parameters. In this study, the printing mechanism of conductive graphene inks with viscosities ranging from 1 to 15 Pa.s using LIFT was investigated. The effects of pulse energy (30 to 120 µJ) and gap distance (50 to 300 μm) in printing voxels with a green nanosecond laser were systematically examined, providing a phenomenological understanding of the material transfer mechanism. The findings highlight the significant role of the temporal pulse distance in enhancing the wet thickness achievable during LIFT of high-viscosity inks, attributed to capillary healing phenomena. Additionally, the acceptor substrates' hydrophobicity was found to increase the wet thickness and improve the resolution of the printed voxels/tracks. Especially, the aspect ratio of LIFT-printed tracks was increased by more than 175% with 10 printing passes when a hydrophobic accepter was used. So, the optimal LIFT processing conditions were identified to achieve high-quality, high-aspect-ratio tracks, by considering synergistically the effects of the temporal pulse distance and the substrate wettability. Moreover, the resistivity of the LIFT-printed graphene tracks decreased by more than 84% after a 100-minute sintering step at 120 °C. This research advances understanding of LIFT printing high-viscosity conductive inks, particularly underpinning the development of high-resolution and high-aspect-ratio electrical circuits for printed electronics. [ABSTRACT FROM AUTHOR] |
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| Database: | Engineering Source |
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| Abstract: | Laser-induced forward transfer (LIFT) is gaining significant attention as a non-contact printing technique for high-viscosity conductive inks in printed electronics. However, the high wet thickness of printed tracks is essential for achieving effective electrical pathways, a requirement that has not been thoroughly considered so far. The wet thickness is a function of ink viscosity, substrate wettability, and the laser processing parameters. In this study, the printing mechanism of conductive graphene inks with viscosities ranging from 1 to 15 Pa.s using LIFT was investigated. The effects of pulse energy (30 to 120 µJ) and gap distance (50 to 300 μm) in printing voxels with a green nanosecond laser were systematically examined, providing a phenomenological understanding of the material transfer mechanism. The findings highlight the significant role of the temporal pulse distance in enhancing the wet thickness achievable during LIFT of high-viscosity inks, attributed to capillary healing phenomena. Additionally, the acceptor substrates' hydrophobicity was found to increase the wet thickness and improve the resolution of the printed voxels/tracks. Especially, the aspect ratio of LIFT-printed tracks was increased by more than 175% with 10 printing passes when a hydrophobic accepter was used. So, the optimal LIFT processing conditions were identified to achieve high-quality, high-aspect-ratio tracks, by considering synergistically the effects of the temporal pulse distance and the substrate wettability. Moreover, the resistivity of the LIFT-printed graphene tracks decreased by more than 84% after a 100-minute sintering step at 120 °C. This research advances understanding of LIFT printing high-viscosity conductive inks, particularly underpinning the development of high-resolution and high-aspect-ratio electrical circuits for printed electronics. [ABSTRACT FROM AUTHOR] |
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| ISSN: | 09478396 |
| DOI: | 10.1007/s00339-025-08433-x |
