High Dynamic Range CsFAPbI 3 Perovskite Photodetectors with 12.7 MHz Bandwidth.

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Title: High Dynamic Range CsFAPbI 3 Perovskite Photodetectors with 12.7 MHz Bandwidth.
Authors: Majeed, Abdul Mannan1 (AUTHOR) gediminas.kreiza@ff.vu.lt, Stanionytė, Sandra2 (AUTHOR), Kreiza, Gediminas1 (AUTHOR), Ščajev, Patrik1,2 (AUTHOR) patrik.scajev@ff.vu.lt
Source: Materials (1996-1944). Apr2026, Vol. 19 Issue 7, p1315. 14p.
Subjects: Photodetectors, Bandwidths, Spin coating, Visible spectra, X-ray diffraction, Imaging systems, Perovskite, Photosensitivity
Abstract: We develop CsxFA1−xPbI3 perovskite photodetectors with varying Cs content in the x = 0.05–0.25 range to identify the most stable cubic-lattice perovskite composition for visible-light photodetection. The perovskite layers were deposited by the spin-coating technique on a nickel oxide p-type contact and then were covered with C60/Ag electron contact to obtain a vertical pin diode structure. X-ray diffraction (XRD) and scanning electron microscopy (SEM) measurements show that x = 0.1–0.2 provides the most stable lattice and pinhole-free perovskite layers. The photocurrents are linear in an extremely wide 1 nW–10 mW excitation power range, providing photoresponsivity of 0.28 A/W at 532 nm (green light), similar to that of Si photodiodes. The testing of the photodetectors using picosecond pulses provided their rise times and fall times. The x = 0.2 composition provided the shortest rise time values of 27.5 ns, leading to a detector modulation bandwidth of 12.7 MHz. This indicates that this perovskite composition is suitable for replacing silicon photodetectors in cost-efficient light detection systems for imaging and light communication applications such as Li-Fi. [ABSTRACT FROM AUTHOR]
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Abstract:We develop CsxFA1−xPbI3 perovskite photodetectors with varying Cs content in the x = 0.05–0.25 range to identify the most stable cubic-lattice perovskite composition for visible-light photodetection. The perovskite layers were deposited by the spin-coating technique on a nickel oxide p-type contact and then were covered with C60/Ag electron contact to obtain a vertical pin diode structure. X-ray diffraction (XRD) and scanning electron microscopy (SEM) measurements show that x = 0.1–0.2 provides the most stable lattice and pinhole-free perovskite layers. The photocurrents are linear in an extremely wide 1 nW–10 mW excitation power range, providing photoresponsivity of 0.28 A/W at 532 nm (green light), similar to that of Si photodiodes. The testing of the photodetectors using picosecond pulses provided their rise times and fall times. The x = 0.2 composition provided the shortest rise time values of 27.5 ns, leading to a detector modulation bandwidth of 12.7 MHz. This indicates that this perovskite composition is suitable for replacing silicon photodetectors in cost-efficient light detection systems for imaging and light communication applications such as Li-Fi. [ABSTRACT FROM AUTHOR]
ISSN:19961944
DOI:10.3390/ma19071315